articleThe Journal of Physical Chemistry CSep 12, 2008Closed access

Functionalization of Halloysite Clay Nanotubes by Grafting with γ-Aminopropyltriethoxysilane

University of Sydney · Guangzhou Institute of Geochemistry · +2 more institutions

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Abstract

Surface modification of natural halloysite clay nanotubes with γ-aminopropyltriethoxysilane (APTES) was investigated. Untreated and modified samples were characterized by nitrogen adsorption, X-ray diffraction, elemental analysis, thermogravimetry, transmission electron microscopy, atomic force microscopy, MAS nuclear magnetic resonance (29Si, 13C, 29Al), and Fourier transform infrared spectroscopy. The modification mechanism was found to include not only the direct grafting of APTES onto the hydroxyl groups of the internal walls, edges and external surfaces of the nanotubes but other processes in which oligomerized APTES condensed with the directly grafted APTES to form a cross-linked structure. The thermal…

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