articleJournal of the American Chemical SocietyJun 11, 2014Closed access

Enhanced Photocatalytic CO 2 -Reduction Activity of Anatase TiO 2 by Coexposed {001} and {101} Facets

Wuhan University of Technology · Kent State University

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Abstract

Control of TiO2 crystal facets has attracted enormous interest due to the fascinating shape-dependent photocatalytic activity of this material. In this work, the effect of the ratio of {001} and {101} facets on the photocatalytic CO2-reduction performance of anatase TiO2 is reported. A new "surface heterojunction" concept is proposed on the basis of the density functional theory (DFT) calculations to explain the difference in the photocatalytic activity of TiO2 with coexposed {001} and {101} facets.

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1,867
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Authors

5

Topics & keywords

Keywords
  • Anatase
  • Photocatalysis
  • Chemistry
  • Heterojunction
  • Reduction (mathematics)
  • Density functional theory
  • Crystal (programming language)
  • Chemical engineering
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