articleProceedings of the National Academy of SciencesAug 27, 2012BRONZE OA

Brown carbon and internal mixing in biomass burning particles

Cooperative Institute for Research in Environmental Sciences · University of Colorado Boulder · +2 more institutions

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Abstract

Biomass burning (BB) contributes large amounts of black carbon (BC) and particulate organic matter (POM) to the atmosphere and contributes significantly to the earth's radiation balance. BB particles can be a complicated optical system, with scattering and absorption contributions from BC, internal mixtures of BC and POM, and wavelength-dependent absorption of POM. Large amounts of POM can also be externally mixed. We report on the unique ability of multi-wavelength photo-acoustic measurements of dry and thermal-denuded absorption to deconstruct this complicated wavelength-dependent system of absorption and mixing. Optical measurements of BB particles from the Four Mile Canyon fire near Boulder, Colorado,…

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