articlePhysical Chemistry Chemical PhysicsJan 1, 2015HYBRID OA

Electrochemical in situ investigations of SEI and dendrite formation on the lithium metal anode

University of Münster · Battery Park

PubMed
Indexed incrossrefpubmed

Abstract

This comparative work studies the self-enforcing heterogeneity of lithium deposition and dissolution as the cause for dendrite formation on the lithium metal anode in various liquid organic solvent based electrolytes. In addition, the ongoing lithium corrosion, its rate and thus the passivating quality of the SEI are investigated in self-discharge measurements. The behavior of the lithium anode is characterized in two carbonate-based standard electrolytes, 1 M LiPF6 in EC/DEC (3 : 7) and 1 M LiPF6 in EC/DMC (1 : 1), and in two alternative electrolytes 1 M LiPF6 in TEGDME and 1 M LiTFSI in DMSO, which have been proposed in the literature as promising electrolytes for lithium metal batteries, more specifically…

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772
total citations
FWCI
29.11
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100%
References
41
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Authors

3

Topics & keywords

Keywords
  • Electrolyte
  • Anode
  • Lithium (medication)
  • Dissolution
  • Electrochemistry
  • Dendrite (mathematics)
  • Inorganic chemistry
  • Chemistry
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