articleJournal of the American Chemical SocietyFeb 13, 2015Closed access

Removal of Interstitial H 2 O in Hexacyanometallates for a Superior Cathode of a Sodium-Ion Battery

The University of Texas at Austin · Stony Brook University · +2 more institutions

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Abstract

Sodium is globally available, which makes a sodium-ion rechargeable battery preferable to a lithium-ion battery for large-scale storage of electrical energy, provided a host cathode for Na can be found that provides the necessary capacity, voltage, and cycle life at the prescribed charge/discharge rate. Low-cost hexacyanometallates are promising cathodes because of their ease of synthesis and rigid open framework that enables fast Na(+) insertion and extraction. Here we report an intriguing effect of interstitial H2O on the structure and electrochemical properties of sodium manganese(II) hexacyanoferrates(II) with the nominal composition Na2MnFe(CN)6·zH2O (Na2-δMnHFC). The newly discovered dehydrated…

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Authors

10

Topics & keywords

Keywords
  • Electrochemistry
  • Chemistry
  • Cathode
  • Anode
  • Battery (electricity)
  • Sodium
  • Lithium (medication)
  • Ion
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