articleAngewandte Chemie International EditionSep 24, 2014Closed access

A Cost‐Effective 3D Hydrogen Evolution Cathode with High Catalytic Activity: FeP Nanowire Array as the Active Phase

Changchun Institute of Applied Chemistry · China West Normal University · +1 more institution

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Abstract

Iron is the cheapest and one of the most abundant transition metals. Natural [FeFe]-hydrogenases exhibit remarkably high activity in hydrogen evolution, but they suffer from high oxygen sensitivity and difficulty in scale-up. Herein, an FeP nanowire array was developed on Ti plate (FeP NA/Ti) from its β-FeOOH NA/Ti precursor through a low-temperature phosphidation reaction. When applied as self-supported 3D hydrogen evolution cathode, the FeP NA/Ti electrode shows exceptionally high catalytic activity and good durability, and it only requires overpotentials of 55 and 127 mV to afford current densities of 10 and 100 mA cm(2) , respectively. The excellent electrocatalytic performance is promising for…

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