articleNature CommunicationsSep 24, 2014HYBRID OA

Combinatorial molecular optimization of cement hydrates

Massachusetts Institute of Technology · Centre National de la Recherche Scientifique · +1 more institution

PubMed
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Abstract

Despite its ubiquitous presence in the built environment, concrete’s molecular-level properties are only recently being explored using experimental and simulation studies. Increasing societal concerns about concrete’s environmental footprint have provided strong motivation to develop new concrete with greater specific stiffness or strength (for structures with less material). Herein, a combinatorial approach is described to optimize properties of cement hydrates. The method entails screening a computationally generated database of atomic structures of calcium-silicate-hydrate, the binding phase of concrete, against a set of three defect attributes: calcium-to-silicon ratio as compositional index and two…

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