Enhanced Singlet Oxygen Generation in Oxidized Graphitic Carbon Nitride for Organic Synthesis
University of Science and Technology of China · Collaborative Innovation Center of Chemistry for Energy Materials · +2 more institutions
Abstract
Experimental data reveal that the incorporation of carbonyl groups into polymer matrix can significantly enhance singlet oxygen (1O2) generation and suppress production of other reactive oxygen species. Excitonic processes investigated by phosphorescence spectroscopy reveal enhanced triplet-exciton generation in the modified g-C3N4, which facilitate 1O2 generation through an energy transfer process. Benefiting from this, the modified g-C3N4 shows excellent conversion and selectivity in organic synthesis. As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not…
Citation impact
- FWCI
- 23.25
- Percentile
- 100%
- References
- 35
Authors
12- HWHui Wang
University of Science and Technology of China, Collaborative Innovation Center of Chemistry for Energy Materials, Quantum Design (Germany)
- SJShenlong Jiang
Collaborative Innovation Center of Chemistry for Energy Materials, Quantum Design (Germany), University of Science and Technology of China
- SCShichuan Chen
Quantum Design (Germany), University of Science and Technology of China, Collaborative Innovation Center of Chemistry for Energy Materials
- DLDandan Li
Anhui University
- XZXiaodong ZhangCorresponding
Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China, Quantum Design (Germany)
Topics & keywords
- Singlet oxygen
- Phosphorescence
- Graphitic carbon nitride
- Materials science
- Organic synthesis
- Photochemistry
- Spectroscopy
- Oxygen
- Affordable and clean energy