Single-atom catalysts for CO 2 electroreduction with significant activity and selectivity improvements
Daejeon University · Korea Advanced Institute of Science and Technology · +1 more institution
Abstract
OH production compared to any existing catalysts, synthesized or predicted. To understand the origin of the activity enhancement of SACs, we find that the lack of an atomic ensemble for adsorbate binding and the unique electronic structure of the single atom catalysts as well as orbital interaction play an important role, contributing to binding energies of SACs that deviate considerably from the conventional scaling relation of bulk transition metals.
Citation impact
- FWCI
- 14.62
- Percentile
- 100%
- References
- 43
Authors
5- SBSeoin Back
Daejeon University, Korea Advanced Institute of Science and Technology
- JLJuhyung Lim
Daejeon University, Korea Advanced Institute of Science and Technology
- NKNa-Young Kim
Daejeon University, Korea Advanced Institute of Science and Technology, Center for NanoScience
- YKYong‐Hyun Kim
Daejeon University, Korea Advanced Institute of Science and Technology, Center for NanoScience
- YJYousung JungCorresponding
Daejeon University, Korea Advanced Institute of Science and Technology
Topics & keywords
- Selectivity
- Catalysis
- Atom (system on chip)
- Chemistry
- Computer science
- Organic chemistry
- Embedded system
Funding
- NRNational Research Foundation
- NRNational Research Foundation of KoreaAwards: NRF-2014H1A2A1016055, NRF-2016M3D1A1021147, NRF-2015R1A2A1A15055539, 2016M3D1A1021147, NRF-2015
- AFAgency for Defense DevelopmentAward: UD140047GD
- KAKorea Advanced Institute of Science and TechnologyAwards: N11160016, EEWS-2016-N11160016