articleAdvanced Functional MaterialsFeb 7, 2017GREEN OA

Cellulose Nanocrystal Inks for 3D Printing of Textured Cellular Architectures

Swiss Federal Laboratories for Materials Science and Technology · ETH Zurich · +2 more institutions

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Abstract

3D printing of renewable building blocks like cellulose nanocrystals offers an attractive pathway for fabricating sustainable structures. Here, viscoelastic inks composed of anisotropic cellulose nanocrystals (CNC) that enable patterning of 3D objects by direct ink writing are designed and formulated. These concentrated inks are composed of CNC particles suspended in either water or a photopolymerizable monomer solution. The shear‐induced alignment of these anisotropic building blocks during printing is quantified by atomic force microscopy, polarized light microscopy, and 2D wide‐angle X‐ray scattering measurements. Akin to the microreinforcing effect in plant cell walls, the alignment of CNC particles during…

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