articleAdvanced MaterialsJun 22, 2017Closed access

High‐Performance 2.6 V Aqueous Asymmetric Supercapacitors based on In Situ Formed Na 0.5 MnO 2 Nanosheet Assembled Nanowall Arrays

Nanjing University of Science and Technology

PubMed
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Abstract

The voltage limit for aqueous asymmetric supercapacitors is usually 2 V, which impedes further improvement in energy density. Here, high Na content Birnessite Na 0.5 MnO 2 nanosheet assembled nanowall arrays are in situ formed on carbon cloth via electrochemical oxidation. It is interesting to find that the electrode potential window for Na 0.5 MnO 2 nanowall arrays can be extended to 0–1.3 V (vs Ag/AgCl) with significantly increased specific capacitance up to 366 F g −1 . The extended potential window for the Na 0.5 MnO 2 electrode provides the opportunity to further increase the cell voltage of aqueous asymmetric supercapacitors beyond 2 V. To construct the asymmetric supercapacitor, carbon‐coated Fe 3 O 4…

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Authors

6

Topics & keywords

Keywords
  • Nanosheet
  • Materials science
  • Supercapacitor
  • In situ
  • Aqueous solution
  • Nanotechnology
  • Chemical engineering
  • Capacitance
UN Sustainable Development Goals
  • Affordable and clean energy
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