articleAdvanced Energy MaterialsJul 21, 2017GREEN OA

“Water‐in‐Salt” Electrolyte Makes Aqueous Sodium‐Ion Battery Safe, Green, and Long‐Lasting

University of Maryland, College Park · DEVCOM Army Research Laboratory · +3 more institutions

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Abstract

Abstract Narrow electrochemical stability window (1.23 V) of aqueous electrolytes is always considered the key obstacle preventing aqueous sodium‐ion chemistry of practical energy density and cycle life. The sodium‐ion water‐in‐salt electrolyte (NaWiSE) eliminates this barrier by offering a 2.5 V window through suppressing hydrogen evolution on anode with the formation of a Na + ‐conducting solid‐electrolyte interphase (SEI) and reducing the overall electrochemical activity of water on cathode. A full aqueous Na‐ion battery constructed on Na 0.66 [Mn 0.66 Ti 0.34 ]O 2 as cathode and NaTi 2 (PO 4 ) 3 as anode exhibits superior performance at both low and high rates, as exemplified by extraordinarily high…

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