articleAdvanced MaterialsFeb 19, 2019Closed access

Achieving Over 15% Efficiency in Organic Photovoltaic Cells via Copolymer Design

Chinese Academy of Sciences · Beijing National Laboratory for Molecular Sciences · +3 more institutions

PubMed
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Abstract

Ternary blending and copolymerization strategies have proven advantageous in boosting the photovoltaic performance of organic solar cells. Here, 15% efficiency solar cells using copolymerization donors are demonstrated, where the electron-withdrawing unit, ester-substituted thiophene, is incorporated into a PBDB-TF polymer to downshift the molecular energy and broaden the absorption. Copolymer-based solar cells suitable for large-area devices can be fabricated by a blade-coating method from a nonhalogen and nonaromatic solvent mixture. Although ternary solar cells can achieve comparable efficiencies, they are not suitable for environment-friendly processing conditions and show relatively low photostability…

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