articleJournal of the American Chemical SocietyJul 26, 2019Closed access

Scalable Production of Efficient Single-Atom Copper Decorated Carbon Membranes for CO 2 Electroreduction to Methanol

Shenzhen University · University of Science and Technology of China · +1 more institution

PubMed
Indexed incrossrefpubmed

Abstract

Electrocatalytic reduction reaction of CO2 (CO2RR) is an effective way to mitigate energy and environmental issues. However, very limited catalysts are capable of converting CO2 resources into high-value products such as hydrocarbons or alcohols. Herein, we first propose a facile strategy for the large-scale synthesis of isolated Cu decorated through-hole carbon nanofibers (CuSAs/TCNFs). This CuSAs/TCNFs membrane has excellent mechanical properties and can be directly used as cathode for CO2RR, which could generate nearly pure methanol with 44% Faradaic efficiency in liquid phase. The self-supporting and through-hole structure of CuSAs/TCNFs greatly reduces the embedded metal atoms and produces abundant…

No related works found for this paper.

Funding