articleAdvanced MaterialsJun 26, 2020Closed access

Mechanically Robust, Elastic, and Healable Ionogels for Highly Sensitive Ultra‐Durable Ionic Skins

Jilin University · State Key Laboratory of Supramolecular Structure and Materials

PubMed
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Abstract

The fabrication of highly durable skin-mimicking sensors remains challenging because of the unavoidable fatigue and physical damage that sensors are subjected to in practical applications. In this study, ultra-durable ionic skins (I-skins) with excellent healability and high sensitivity are fabricated by impregnating ionic liquids (ILs) into a mechanically robust poly(urea-urethane) (PU) network. The PU network is composed of crystallized poly(ε-caprolactone) and flexible poly(ethylene glycol) that are dynamically cross-linked with hindered urea bonds and hydrogen bonds. Such a design endows the resultant ionogels with high mechanical strength, good elasticity, Young's modulus similar to that of natural skin,…

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