articleAdvanced MaterialsJul 12, 2020Closed access

Directly Grown Vertical Graphene Carpets as Janus Separators toward Stabilized Zn Metal Anodes

Soochow University · State Key Laboratory of New Ceramics and Fine Processing · +3 more institutions

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Abstract

Abstract Zinc metal anode has garnered a great deal of scientific and technological interest. Nevertheless, major bottlenecks restricting its large‐scale utilization lie in the poor electrochemical stability and unsatisfactory cycling life. Herein, a Janus separator is developed via directly growing vertical graphene (VG) carpet on one side of commercial glass fiber separator throughout chemical vapor deposition. A simple air plasma treatment further renders the successful incorporation of oxygen and nitrogen heteroatoms on bare graphene. Thus‐derived 3D VG scaffold affording large surface area and porous structure can be viewed as a continuation of planar zinc anode. In turn, the Janus separator harvests…

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