Interface Issues and Challenges in All‐Solid‐State Batteries: Lithium, Sodium, and Beyond

Owing to the promise of high safety and energy density, all-solid-state batteries are attracting incremental interest as one of the most promising next-generation energy storage systems. However, their widespread applications are inhibited by many technical challenges, including low-conductivity electrolytes, dendrite growth, and poor cycle/rate properties. Particularly, the interfacial dynamics between the solid electrolyte and the electrode is considered as a crucial factor in determining solid-state battery performance. In recent years, intensive research efforts have been devoted to understanding the interfacial behavior and strategies to overcome these challenges for all-solid-state batteries. Here, the…

• NN
  National Natural Science Foundation of China

  Awards: 21905071, 51773049
• HI
  Harbin Institute of Technology