articleJournal of the American Chemical SocietyFeb 9, 2022Closed access

A Covalent Organic Framework/Graphene Dual-Region Hydrogel for Enhanced Solar-Driven Water Generation

University of Vienna · Technische Universität Berlin · +2 more institutions

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Abstract

Solar-driven water generation is a sustainable water treatment technology, helping to relieve global water scarcity issues. However, this technology faces great challenges due to the high energy consumption of water evaporation yielding low evaporation rates. Here, a covalent organic framework (COF)/graphene dual-region hydrogel, containing hydrophilic and hydrophobic regions in one material, is developed through a facile in situ growth strategy. The hydrophilic COF is covering parts of the hydrophobic graphene regions. Through accurate control of both wetting regions, the hybrid hydrogel shows effective light-harvesting, tunable wettability, optimized water content, and lowered energy demand for water…

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