articleAdvanced Functional MaterialsFeb 9, 2022Closed access

A Universal Strategy toward Air‐Stable and High‐Rate O3 Layered Oxide Cathodes for Na‐Ion Batteries

Fujian Normal University · Chinese Academy of Sciences · +2 more institutions

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Abstract

Abstract As one of the fascinating high capacity cathodes, O3‐type layered oxides usually suffer from their intrinsic air sensitivity and sluggish kinetics originating from the spontaneous lattice Na extraction during air exposure and high tetrahedral site energy of Na + diffusion transition state. What is worse, the improvement on the two handicaps is hard to simultaneously realize because of the contradiction between Na containment suggested in air stability mechanism and enhanced Na diffusion mentioned in kinetics strategy. Herein, it is shown that a simple strategy of introducing proper Na vacancies into lattice can simultaneously realize a dual performance improvement. Na vacancies decrease the charge…

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235
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FWCI
19.57
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100%
References
55
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Authors

11

Topics & keywords

Keywords
  • Materials science
  • Cathode
  • Lattice (music)
  • Ion
  • Oxide
  • Diffusion barrier
  • Kinetics
  • Chemical physics
UN Sustainable Development Goals
  • Affordable and clean energy
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