articleScienceMay 12, 2022Closed access

Scalable processing for realizing 21.7%-efficient all-perovskite tandem solar modules

Collaborative Innovation Center of Advanced Microstructures · Nanjing University · +3 more institutions

PubMed
Indexed incrossrefpubmed

Abstract

Challenges in fabricating all-perovskite tandem solar cells as modules rather than as single-junction configurations include growing high-quality wide-bandgap perovskites and mitigating irreversible degradation caused by halide and metal interdiffusion at the interconnecting contacts. We demonstrate efficient all-perovskite tandem solar modules using scalable fabrication techniques. By systematically tuning the cesium ratio of a methylammonium-free 1.8-electron volt mixed-halide perovskite, we improve the homogeneity of crystallization for blade-coated films over large areas. An electrically conductive conformal "diffusion barrier" is introduced between interconnecting subcells to improve the power conversion…

Citation impact

311
total citations
FWCI
26.22
Percentile
100%
References
48
Citations per year

Authors

15

Topics & keywords

Keywords
  • Tandem
  • Perovskite (structure)
  • Materials science
  • Energy conversion efficiency
  • Optoelectronics
  • Fabrication
  • Halide
  • Band gap
UN Sustainable Development Goals
  • Affordable and clean energy
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