articleNature CommunicationsJun 10, 2022GOLD OA

Converting waste PET plastics into automobile fuels and antifreeze components

Yunnan Institute of Environmental Sciences · East China Normal University · +1 more institution

PubMed
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Abstract

Abstract With the aim to solve the serious problem of white plastic pollution, we report herein a low-cost process to quantitatively convert polyethylene terephthalate (PET) into p -xylene (PX) and ethylene glycol (EG) over modified Cu/SiO 2 catalyst using methanol as both solvent and hydrogen donor. Kinetic and in-situ Fourier-transform infrared spectroscopy (FTIR) studies demonstrate that the degradation of PET into PX involves tandem PET methanolysis and dimethyl terephthalate (DMT) selective hydro-deoxygenation (HDO) steps with the in-situ produced H 2 from methanol decomposition at 210 °C. The overall high activities are attributed to the high Cu + /Cu 0 ratio derived from the dense and granular copper…

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