articleAdvanced MaterialsJul 15, 2022Closed access

A New Polymer Donor Enables Binary All‐Polymer Organic Photovoltaic Cells with 18% Efficiency and Excellent Mechanical Robustness

Chinese Academy of Sciences · Beijing National Laboratory for Molecular Sciences · +4 more institutions

PubMed
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Abstract

The development of polymerized small-molecule acceptors has boosted the power conversion efficiencies (PCEs) of all-polymer organic photovoltaic (OPV) cells to 17%. However, the polymer donors suitable for all-polymer OPV cells are still lacking, restricting the further improvement of their PCEs. Herein, a new polymer donor named PQM-Cl is designed and its photovoltaic performance is explored. The negative electrostatic potential and low average local ionization energy distribution of the PQM-Cl surface enable efficient charge generation and transfer process. When blending with a well-used polymer acceptor, PY-IT, the PQM-Cl-based devices deliver an impressive PCE of 18.0% with a superior fill factor of 80.7%,…

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