articleAccounts of Chemical ResearchSep 26, 2022Closed access

Thermo-, Electro-, and Photocatalytic CO 2 Conversion to Value-Added Products over Porous Metal/Covalent Organic Frameworks

Chinese Academy of Sciences · Fujian Institute of Research on the Structure of Matter · +3 more institutions

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Abstract

ConspectusThe continuing increase of the concentration of atmospheric CO2 has caused many environmental issues including climate change. Catalytic conversion of CO2 using thermochemical, electrochemical, and photochemical methods is a potential technique to decrease the CO2 concentration and simultaneously obtain value-added chemicals. Due to the high energy barrier of CO2 however, this method is still far from large-scale applications which requires high activity, selectivity, and stability. Therefore, development of efficient catalysts to convert CO2 to different products is urgent. With their well-engineered pores and chemical compositions, high surface area, elevated CO2 adsorption capability, and…

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