articleNature CommunicationsJan 10, 2023GOLD OA

Vascular smooth muscle-inspired architecture enables soft yet tough self-healing materials for durable capacitive strain-sensor

Nanjing Forestry University · Nanjing University of Science and Technology · +2 more institutions

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Abstract

Abstract Catastrophically mechanical failure of soft self-healing materials is unavoidable due to their inherently poor resistance to crack propagation. Here, with a model system, i.e., soft self-healing polyurea, we present a biomimetic strategy of surpassing trade-off between soft self-healing and high fracture toughness, enabling the conversion of soft and weak into soft yet tough self-healing material. Such an achievement is inspired by vascular smooth muscles, where core-shell structured Galinstan micro-droplets are introduced through molecularly interfacial metal-coordinated assembly, resulting in an increased crack-resistant strain and fracture toughness of 12.2 and 34.9 times without sacrificing…

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