articleNature CommunicationsFeb 15, 2023GOLD OA

One-stone-for-two-birds strategy to attain beyond 25% perovskite solar cells

Ministry of Education of the People's Republic of China · Advanced Energy Materials (United States) · +7 more institutions

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Abstract

Even though the perovskite solar cell has been so popular for its skyrocketing power conversion efficiency, its further development is still roadblocked by its overall performance, in particular long-term stability, large-area fabrication and stable module efficiency. In essence, the soft component and ionic-electronic nature of metal halide perovskites usually chaperonage large number of anion vacancy defects that act as recombination centers to decrease both the photovoltaic efficiency and operational stability. Herein, we report a one-stone-for-two-birds strategy in which both anion-fixation and associated undercoordinated-Pb passivation are in situ achieved during crystallization by using a single…

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