articleNature CommunicationsFeb 22, 2023GOLD OA

Synergistic promotions between CO2 capture and in-situ conversion on Ni-CaO composite catalyst

East China University of Science and Technology · State Key Laboratory of Chemical Engineering · +1 more institution

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Abstract

Abstract The integrated CO 2 capture and conversion (iCCC) technology has been booming as a promising cost-effective approach for Carbon Neutrality. However, the lack of the long-sought molecular consensus about the synergistic effect between the adsorption and in-situ catalytic reaction hinders its development. Herein, we illustrate the synergistic promotions between CO 2 capture and in-situ conversion through constructing the consecutive high-temperature Calcium-looping and dry reforming of methane processes. With systematic experimental measurements and density functional theory calculations, we reveal that the pathways of the reduction of carbonate and the dehydrogenation of CH 4 can be interactively…

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