articleNature CommunicationsFeb 27, 2023GOLD OA

Polyamide membranes with nanoscale ordered structures for fast permeation and highly selective ion-ion separation

China Agricultural University · National University of Singapore · +2 more institutions

PubMed
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Abstract

Abstract Fast permeation and effective solute-solute separation provide the opportunities for sustainable water treatment, but they are hindered by ineffective membranes. We present here the construction of a nanofiltration membrane with fast permeation, high rejection, and precise Cl - /SO 4 2- separation by spatial and temporal control of interfacial polymerization via graphitic carbon nitride (g-C 3 N 4 ). The g-C 3 N 4 nanosheet binds preferentially with piperazine and tiles the water-hexane interface as revealed by molecular dynamics studies, thus lowering the diffusion rate of PIP by one order of magnitude and restricting its diffusion pathways towards the hexane phase. As a result, membranes with…

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251
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Authors

10

Topics & keywords

Keywords
  • Permeation
  • Membrane
  • Nanofiltration
  • Permeance
  • Interfacial polymerization
  • Materials science
  • Chemical engineering
  • Molecular dynamics
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