articleNature CommunicationsMar 18, 2023GOLD OA

Mesoporous Pt@Pt-skin Pt3Ni core-shell framework nanowire electrocatalyst for efficient oxygen reduction

Wuhan University of Technology · University of Namur · +1 more institution

PubMed
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Abstract

Abstract The design of Pt-based nanoarchitectures with controllable compositions and morphologies is necessary to enhance their electrocatalytic activity. Herein, we report a rational design and synthesis of anisotropic mesoporous Pt@Pt-skin Pt 3 Ni core-shell framework nanowires for high-efficient electrocatalysis. The catalyst has a uniform core-shell structure with an ultrathin atomic-jagged Pt nanowire core and a mesoporous Pt-skin Pt 3 Ni framework shell, possessing high electrocatalytic activity, stability and Pt utilisation efficiency. For the oxygen reduction reaction, the anisotropic mesoporous Pt@Pt-skin Pt 3 Ni core-shell framework nanowires demonstrated exceptional mass and specific activities of…

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213
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100%
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Authors

17

Topics & keywords

Keywords
  • Electrocatalyst
  • Mesoporous material
  • Nanowire
  • Materials science
  • Catalysis
  • Nanotechnology
  • Chemical engineering
  • Electrode
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