articleNature PhotonicsMay 8, 2023HYBRID OA

Stable perovskite single-crystal X-ray imaging detectors with single-photon sensitivity

ETH Zurich · Swiss Federal Laboratories for Materials Science and Technology · +1 more institution

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Abstract

Abstract A major thrust of medical X-ray imaging is to minimize the X-ray dose acquired by the patient, down to single-photon sensitivity. Such characteristics have been demonstrated with only a few direct-detection semiconductor materials such as CdTe and Si; nonetheless, their industrial deployment in medical diagnostics is still impeded by elaborate and costly fabrication processes. Hybrid lead halide perovskites can be a viable alternative owing to their facile solution growth. However, hybrid perovskites are unstable under high-field biasing in X-ray detectors, owing to structural lability and mixed electronic–ionic conductivity. Here we show that both single-photon-counting and long-term stable…

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