Intermetallic Single-Atom Alloy In–Pd Bimetallene for Neutral Electrosynthesis of Ammonia from Nitrate
Walker (United States) · The University of Texas at Austin · +3 more institutions
Abstract
Harvesting recyclable ammonia (NH3) from the electrocatalytic reduction of nitrate (NO3RR) offers a sustainable strategy to close the ecological nitrogen cycle from nitration contamination in an energy-efficient and environmentally friendly manner. The emerging intermetallic single-atom alloys (ISAAs) are recognized to achieve the highest site density of single atoms by isolating contiguous metal atoms into single sites stabilized by another metal within the intermetallic structure, which holds promise to couple the catalytic benefits from intermetallic nanocrystals and single-atom catalysts for promoting NO3RR. Herein, ISAA In–Pd bimetallene, in which the Pd single atoms are isolated by surrounding In atoms,…
Citation impact
- FWCI
- 17.93
- Percentile
- 100%
- References
- 61
Authors
9- MXMinghao Xie
Walker (United States), The University of Texas at Austin
- STSishuang Tang
Walker (United States), The University of Texas at Austin
- LZLi Zhao
Walker (United States), The University of Texas at Austin
- MWMaoyu Wang
Argonne National Laboratory
- ZJZhaoyu Jin
University of Electronic Science and Technology of China
Topics & keywords
- Electrosynthesis
- Chemistry
- Intermetallic
- Nitrate
- Alloy
- Ammonia
- Ammonia production
- Inorganic chemistry
- Responsible consumption and production
Funding
- UDU.S. Department of EnergyAwards: DE-SC0019019, AC02-06CH11357, DE-AC02, 06CH11357, DE-AC02-06CH11357, DE-AC02-
- WFWelch FoundationAward: F-1861
- CACamille and Henry Dreyfus Foundation
- OOOffice of ScienceAwards: DE-AC02-06CH11357, DE-AC02, 06CH11357, AC02-06CH11357
- BEBasic Energy SciencesAwards: DE-AC02, DE-SC0019019, AC02-06CH11357, 06CH11357
- ANArgonne National LaboratoryAwards: DE-AC02, 06CH11357, AC02-06CH11357