articleSmallJul 24, 2023Closed access

Stabilizing Zn Metal Anode Through Regulation of Zn Ion Transfer and Interfacial Behavior with a Fast Ion Conductor Protective Layer

North China University of Science and Technology · Donghua University · +4 more institutions

PubMed
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Abstract

Abstract Aqueous Zn‐ion batteries (AZIBs) attract intensive attention owing to their environmental friendliness, cost‐effectiveness, innate safety, and high specific capacity. However, the practical applications of AZIBs are hindered by several adverse phenomena, including corrosion, Zn dendrites, and hydrogen evolution. Herein, a Zn anode decorated with a 3D porous‐structured Na 3 V 2 (PO4) 3 (NVP@Zn) is obtained, where the NVP reconstruct the electrolyte/anode interface. The resulting NVP@Zn anode can provide a large quantity of fast and stable channels, facilitating enhanced Zn ion deposition kinetics and regulating the Zn ions transport process through the ion confinement effect. The NASICON‐type NVP…

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