articleAdvanced MaterialsJan 5, 2024Closed access

Polymer Molecules Adsorption‐Induced Zincophilic‐Hydrophobic Protective Layer Enables Highly Stable Zn Metal Anodes

Energy Research Institute · South China University of Technology · +1 more institution

PubMed
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Abstract

Abstract Zn metal, as one of the most promising anode materials for aqueous batteries, suffers from uncontrollable dendrite growth and water‐induced parasitic reactions, which drastically compromise its cycle life and Coulombic efficiency (CE). Herein, a nonionic amphipathic additive Tween‐20 (TW20) is proposed that bears both zincophilic and hydrophobic units. The zincophilic segment of TW20 preferentially adsorbs on the Zn anode, while the hydrophobic segment is exposed on the electrolyte side, forming an electrolyte‐facing hydrophobic layer that shields the anode from active water molecules. Moreover, theoretical calculation and experimental results reveal that the TW20 additive can induce the preferential…

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