Microwave‐Assisted Rapid Synthesis of MOF‐Based Single‐Atom Ni Catalyst for CO 2 Electroreduction at Ampere‐Level Current
University of Science and Technology of China · Zhengzhou University · +1 more institution
Abstract
Abstract Carbon‐based single‐atom catalysts (SACs) have attracted tremendous interest in heterogeneous catalysis. However, the common electric heating techniques to produce carbon‐based SACs usually suffer from prolonged heating time and tedious operations. Herein, a general and facile microwave‐assisted rapid pyrolysis method is developed to afford carbon‐based SACs within 3 min without inert gas protection. The obtained carbon‐based SACs present high porosity and comparable carbonization degree to those obtained by electric heating techniques. Specifically, the single‐atom Ni implanted N‐doped carbon (Ni 1 −N−C) derived from a Ni‐doped metal–organic framework (Ni‐ZIF‐8) exhibits remarkable CO Faradaic…
Citation impact
- FWCI
- 12.33
- Percentile
- 100%
- References
- 68
Authors
5- MWMing Wen
University of Science and Technology of China, Zhengzhou University, Hefei National Center for Physical Sciences at Nanoscale
- NSNana Sun
University of Science and Technology of China, Hefei National Center for Physical Sciences at Nanoscale
- LJLong JiaoCorresponding
University of Science and Technology of China, Hefei National Center for Physical Sciences at Nanoscale
- SZShuang‐Quan ZangCorresponding
Zhengzhou University
- HJHai‐Long JiangCorresponding
University of Science and Technology of China, Hefei National Center for Physical Sciences at Nanoscale
Topics & keywords
- Catalysis
- Ampere
- Current (fluid)
- Microwave
- Atom (system on chip)
- Materials science
- Analytical Chemistry (journal)
- Chemistry