articleJournal of the American Chemical SocietyMar 8, 2024Closed access

Hg 4 (Te 2 O 5 )(SO 4 ): A Giant Birefringent Sulfate Crystal Triggered by a Highly Selective Cation

Chinese Academy of Sciences · Fujian Institute of Research on the Structure of Matter · +2 more institutions

PubMed
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Abstract

Sulfate crystals are often criticized for their low birefringence. The small anisotropic SO4 group is becoming the biggest bottleneck hindering the application of sulfates in optical functional materials. In this study, we report a new method to significantly enhance the birefringence of sulfates. The title compound increases the birefringence recording of sulfates to 0.542@546 nm, which is significantly larger than that of the commercial birefringent crystal of TiO2 (0.306@546.1 nm). At the infrared wavelength, the birefringence of Hg4(Te2O5)(SO4) can be up to 0.400@1064 nm, which is also much larger than the infrared birefringent crystal of YVO4 (0.209@1064 nm). In addition, it also has a wide transparency…

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