articleACS CatalysisMar 26, 2024Closed access

Electro-Reforming of PET Plastic to C 2 Chemicals with Concurrent Generation of Hydrogen and Electric Energy

Tongji University · State Key Laboratory of Pollution Control and Resource Reuse · +1 more institution

Indexed incrossref

Abstract

Upcycling poly(ethylene terephthalate) (PET) waste into valuable C2 products presents an alternative avenue for attaining carbon neutrality. In this study, we introduce a C–C preserved pathway for selectively transforming waste PET-derived ethylene glycol (EG) into glycolic acid (GA), a 25-fold value of C2 product. Utilizing a Pt–Ni(OH)2/NF electrode, EG oxidation reaction (EGOR) proceeds at a remarkably low potential (100 mA cm–2 @0.69 V vs reversible hydrogen electrode (RHE)) with an impressive Faraday efficiency (93%) for GA production. In situ Fourier transform infrared (FTIR) measurements are employed to pinpoint crucial reaction intermediates, elucidating C2 pathways for the conversion of EG to GA. Quasi…

Citation impact

148
total citations
FWCI
39.24
Percentile
100%
References
40
Citations per year

Authors

9

Topics & keywords

Keywords
  • Hydrogen production
  • Catalysis
  • Hydrogen
  • Steam reforming
  • Materials science
  • Hydrogen fuel
  • Energy (signal processing)
  • Chemistry
UN Sustainable Development Goals
  • Affordable and clean energy
No related works found for this paper.

Funding