articleAdvanced MaterialsApr 8, 2024BRONZE OA

Water‐Stable High‐Entropy Metal‐Organic Framework Nanosheets for Photocatalytic Hydrogen Production

Dalian Maritime University · Dalian Institute of Chemical Physics · +3 more institutions

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Abstract

Abstract Metal‐organic frameworks (MOFs) have emerged as promising platforms for photocatalytic hydrogen evolution reaction (HER) due to their fascinating physiochemical properties. Rationally engineering the compositions and structures of MOFs can provide abundant opportunities for their optimization. In recent years, high‐entropy materials (HEMs) have demonstrated great potential in the energy and environment fields. However, there is still no report on the development of high‐entropy MOFs (HE‐MOFs) for photocatalytic HER in aqueous solution. Herein, the authors report the synthesis of a novel p ‐type HE‐MOFs single crystal (HE‐MOF‐SC) and the corresponding HE‐MOFs nanosheets (HE‐MOF‐NS) capable of realizing…

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