articleAdvanced Functional MaterialsApr 9, 2024Closed access

3D Ternary Alloy Artificial Interphase Toward Ultra‐Stable and Dendrite‐Free Aqueous Zinc Batteries

North China Electric Power University · Shanxi Normal University

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Abstract

Abstract Rechargeable aqueous zinc‐ion batteries (AZIBs) are one of the most promising post‐lithium battery technologies due to their low cost, high safety, and environmental friendliness. However, their practical development is hindered by the issues of Zn metal anodes, including dendrite growth, passivation, hydrogen evolution and other side reactions. Herein, to circumvent these issues, a facile and universal alloy electrodeposition strategy is proposed to construct a 3D structured ternary Zn alloy artificial interphase layer on Zn foil as an anode for high‐performance AZIBs. The density functional theory (DFT) theoretical calculations, in situ optical visualization and spectroscopic results validate that…

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