Regulating the Topology of Covalent Organic Frameworks for Boosting Overall H 2 O 2 Photogeneration
Shandong Normal University · Ministry of Education · +3 more institutions
Abstract
Abstract Photocatalytic oxygen reduction reactions and water oxidation reactions are extremely promising green approaches for massive H 2 O 2 production. Nonetheless, constructing effective photocatalysts for H 2 O 2 generation is critical and still challenging. Since the network topology has significant impacts on the electronic properties of two dimensional (2D) polymers, herein, for the first time, we regulated the H 2 O 2 photosynthetic activity of 2D covalent organic frameworks (COFs) by topology. Through designing the linking sites of the monomers, we synthesized a pair of novel COFs with similar chemical components on the backbones but distinct topologies. Without sacrificial agents, TBD‐COF with cpt…
Citation impact
- FWCI
- 15.30
- Percentile
- 100%
- References
- 54
Authors
7- JYJieyu Yue
Shandong Normal University, Ministry of Education
- JLJing‐Xian Luo
Shandong Normal University, Ministry of Education
- ZPZi‐Xian Pan
Shandong Normal University, Ministry of Education
- RZRuizhi Zhang
Shandong Normal University, Ministry of Education
- PYPeng Yang
Shandong Normal University, Ministry of Education
Topics & keywords
- Boosting (machine learning)
- Covalent bond
- Photochemistry
- Chemistry
- Topology (electrical circuits)
- Materials science
- Organic chemistry
- Computer science
- Affordable and clean energy