Efficient Photocatalytic CO 2 Reduction in Ellagic Acid–Based Covalent Organic Frameworks
Chinese Academy of Sciences · Fujian Institute of Research on the Structure of Matter · +3 more institutions
Abstract
Employing covalent organic frameworks (COFs) for the photocatalytic CO2 reduction reaction (CDRR) to generate high-value chemical fuels and mitigate greenhouse gas emissions represents a sustainable catalytic conversion approach. However, achieving superior photocatalytic CDRR performance is hindered by the challenges of low charge separation efficiency, poor stability, and high preparation costs associated with COFs. Herein, in this work, we utilized perfluorinated metallophthalocyanine (MPcF16) and the organic biomolecule compound ellagic acid (EA) as building blocks to actualize functional covalent organic frameworks (COFs) named EPM-COF (M = Co, Ni, Cu). The designed EPCo-COF, featuring cobalt metal active…
Citation impact
- FWCI
- 15.95
- Percentile
- 100%
- References
- 45
Authors
6- WLWan Lin
Chinese Academy of Sciences, Fujian Institute of Research on the Structure of Matter, University of Chinese Academy of Sciences
- FLFu‐Wen Lin
Fujian Normal University, Chinese Academy of Sciences, Fujian Institute of Research on the Structure of Matter
- JLJing Lin
Chinese Academy of Sciences, Fujian Institute of Research on the Structure of Matter, Tan Kah Kee Innovation Laboratory
- ZXZhiwei Xiao
Fujian Normal University, Chinese Academy of Sciences, Fujian Institute of Research on the Structure of Matter
- DYDaqiang Yuan
Chinese Academy of Sciences, Fujian Institute of Research on the Structure of Matter, Tan Kah Kee Innovation Laboratory, University of Chinese Academy of Sciences
Topics & keywords
- Chemistry
- Ellagic acid
- Photocatalysis
- Covalent bond
- Reduction (mathematics)
- Organic chemistry
- Combinatorial chemistry
- Environmental chemistry
Funding
- NNNational Natural Science Foundation of ChinaAwards: 22022110, 22279141
- NSNatural Science Foundation of Fujian ProvinceAward: 2022J05094
- NKNational Key Research and Development Program of ChinaAward: 2021YFA1501500
- KRKey Research Program of Frontier Science, Chinese Academy of SciencesAward: ZDBS-LY-SLH028
- FSFujian Science and Technology Innovation Laboratory for Optoelectronic Information of ChinaAwards: 2021ZR123, 2021ZZ106