articleNature CommunicationsJun 19, 2024GOLD OA

High-entropy relaxor ferroelectric ceramics for ultrahigh energy storage

Chinese Academy of Sciences · Shanghai Institute of Ceramics · +3 more institutions

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Abstract

Abstract Dielectric ceramic capacitors with ultrahigh power densities are fundamental to modern electrical devices. Nonetheless, the poor energy density confined to the low breakdown strength is a long-standing bottleneck in developing desirable dielectric materials for practical applications. In this instance, we present a high-entropy tungsten bronze-type relaxor ferroelectric achieved through an equimolar-ratio element design, which realizes a giant recoverable energy density of 11.0 J·cm −3 and a high efficiency of 81.9%. Moreover, the atomic-scale microstructural study confirms that the excellent comprehensive energy storage performance is attributed to the increased atomic-scale compositional…

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