reviewChemical Society ReviewsJan 1, 2024Closed access

Recent advances in zinc-ion dehydration strategies for optimized Zn–metal batteries

City University of Hong Kong, Shenzhen Research Institute · Collaborative Innovation Center of Advanced Microstructures · +3 more institutions

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Abstract

Aqueous Zn-metal batteries have attracted increasing interest for large-scale energy storage owing to their outstanding merits in terms of safety, cost and production. However, they constantly suffer from inadequate energy density and poor cycling stability due to the presence of zinc ions in the fully hydrated solvation state. Thus, designing the dehydrated solvation structure of zinc ions can effectively address the current drawbacks of aqueous Zn-metal batteries. In this case, considering the lack of studies focused on strategies for the dehydration of zinc ions, herein, we present a systematic and comprehensive review to deepen the understanding of zinc-ion solvation regulation. Two fundamental design…

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