articleAdvanced MaterialsJul 25, 2024Closed access

Large Orientation Angle Buried Substrate Enables Efficient Flexible Perovskite Solar Cells and Modules

Chinese Academy of Sciences · University of Chinese Academy of Sciences · +2 more institutions

PubMed
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Abstract

Abstract Flexible perovskite solar cells (f‐PSCs) have emerged as potential candidates for specific mechanical applications owing to their high foldability, efficiency, and portability. However, the power conversion efficiency (PCE) of f‐PSC remains limited by the inferior contact between perovskite and flexible buried substrate. Here, an asymmetric π‐extended self‐assembled monolayer (SAM) (4‐(9H‐dibenzo[a,c]carbazol‐9‐yl)butyl)phosphonic acid (A‐4PADCB) is reported as a buried substrate for efficient inverted f‐PSCs. Employing this design strategy, A‐4PADCB exhibits a significant orientation angle away from the surface normal, homogenizing the distribution of contact potentials. This enhancement improves the…

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