articleAccounts of Chemical ResearchAug 6, 2024Closed access

Electronic Structure and Functions of Carbon Nitride in Frontier Green Catalysis

The University of Adelaide · Ludwig-Maximilians-Universität München · +1 more institution

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Abstract

ConspectusGraphitic carbon nitride-based materials have emerged as promising photocatalysts for a variety of energy and environmental applications owing to their “earth-abundant” nature, structural versatility, tunable electronic and optical properties, and chemical stability. Optimizing carbon nitride’s physicochemical properties encompasses a variety of approaches, including the regulation of inherent structural defects, morphology control, heterostructure construction, and heteroatom and metal-atom doping. These strategies are pivotal in ultimately enhancing their photocatalytic activities. Previous reviews with extensive examples have mainly focused on the synthesis, modification, and application of carbon…

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