Tracking the correlation between spintronic structure and oxygen evolution reaction mechanism of cobalt-ruthenium-based electrocatalyst
Dalian University of Technology · Dalian University · +3 more institutions
Abstract
Regulating the spintronic structure of electrocatalysts can improve the oxygen evolution reaction performance efficiently. Nonetheless, the effects of tuning the spintronic structure for the oxygen evolution reaction mechanisms have rarely been discussed. Here, we show a ruthenium-cobalt-tin oxide with optimized spintronic structure due to the quantum spin interaction of Ru and Co. The specific spintronic structure of ruthenium-cobalt-tin oxide promotes the charge transfer kinetics and intermediates evolution behavior under applied potential, generating long-lived active species with higher spin density sites for the oxygen evolution reaction after the reconstruction process. Moreover, the ruthenium-cobalt-tin…
Citation impact
- FWCI
- 14.05
- Percentile
- 100%
- References
- 70
Authors
10Topics & keywords
- Spintronics
- Oxygen evolution
- Ruthenium
- Cobalt
- Materials science
- Electrocatalyst
- Electron transfer
- Tin