articleNature CommunicationsJan 4, 2025GOLD OA

Hierarchically aligned heterogeneous core-sheath hydrogels

Hefei University of Technology · University of Science and Technology of China · +2 more institutions

PubMed
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Abstract

Natural materials with highly oriented heterogeneous structures are often lightweight but strong, stiff but tough and durable. Such an integration of diverse incompatible mechanical properties is highly desired for man-made materials, especially weak hydrogels which are lack of high-precision structural design. Herein, we demonstrate the fabrication of hierarchically aligned heterogeneous hydrogels consisting of a compactly crosslinked sheath and an aligned porous core with alignments of nanofibrils at multi-scales by a sequential self-assembly assisted salting out method. The produced hydrogel offers ultrahigh mechanical properties among the reported hydrogels, elastomers and natural materials, including a…

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