articleJournal of the American Chemical SocietyJan 14, 2025Closed access

Rational Design of Prussian Blue Analogues for Ultralong and Wide-Temperature-Range Sodium-Ion Batteries

Shandong University · State Key Laboratory of Crystal Materials

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Abstract

Architecting Prussian blue analogue (PBA) cathodes with optimized synergistic bimetallic reaction centers is a paradigmatic strategy for devising high-energy sodium-ion batteries (SIBs); however, these cathodes usually suffer from fast capacity fading and sluggish reaction kinetics. To alleviate the above problems, herein, a series of early transition metal (ETM)–late transition metal (LTM)-based PBA (Fe-VO, Fe-TiO, Fe-ZrO, Co-VO, and Fe-Co-VO) cathode materials have been conveniently fabricated via an “acid-assisted synthesis” strategy. As a paradigm, the FeVO-PBA (FV) delivers a superb rate capability (148.9 and 56.1 mAh/g under 0.5 and 100 C, respectively), remarkable cycling stability over 30,000 cycles,…

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