articleACS NanoFeb 4, 2025Closed access

Boosting Capacitive Deionization in MoS 2 via Interfacial Coordination Bonding and Intercalation-Induced Spacing Confinement

Energy Institute · Southern University of Science and Technology

PubMed
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Abstract

Capacitive deionization (CDI) is a green and promising technology for seawater desalination, with its capacity and industrial application being severely hindered by efficient electrode materials. Layered molybdenum disulfide (MoS2) has garnered significant attention for CDI applications, while its performance is hampered by weak surface hydrophilicity, high interfacial resistance, and sluggish electron transport. Herein, we introduce an interfacial and intercalation dual-engineering strategy by covalently functionalizing the hydrophilic pyridine groups within the 1T-MoS2 layer (Py-MoS2); an electron-rich interface with an expanded interlayer spacing has been achieved synergistically. A state-of-the-art high…

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