articleAngewandte Chemie International EditionFeb 5, 2025Closed access

Integrating Two Photochromics into One Three‐Dimensional Covalent Organic Framework for Synergistically Enhancing Multiple Photocatalytic Oxidations

Shandong University of Technology · Shandong University · +2 more institutions

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Abstract

Abstract While photocatalytic oxidations are a category of important reactions in wide chemical synthesis, the fabrication of effective photocatalysts for broad oxidation reactions is still of a great challenge. Herein, by rationally integrating two photochromics, porphyrin and triphenylamine, a three‐dimensional photoactive covalent organic framework (COF) is successfully constructed for photocatalytic oxidations. Characterization studies not only show the formation of a crystalline and three‐dimensional porous framework, but also reveal its effective photochemical semiconductor properties derived from the porphyrin and triphenylamine moieties. Electron paramagnetic resonance measurements indicate that the…

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52
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100%
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Authors

9

Topics & keywords

Keywords
  • Photocatalysis
  • Triphenylamine
  • Photochemistry
  • Singlet oxygen
  • Covalent bond
  • Alkylbenzenes
  • Porphyrin
  • Covalent organic framework
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