articleAngewandte Chemie International EditionFeb 20, 2025Closed access

Towards Ultra‐Stable Wide‐Temperature Zinc‐Ion Batteries by Using Ion‐Sieving Organic Framework Membrane

Fudan University · Collaborative Innovation Center of Chemistry for Energy Materials · +1 more institution

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Abstract

Abstract Aqueous zinc‐ion batteries (AZIBs) offer notable advantages in safety and cost‐efficiency, but Zn dendrite growth and unstable interfacial reactions hinder their commercial viability. A crucial factor in addressing these challenges lies in optimizing the separator to regulate ion transport and stabilize electrode interfaces. Herein, we propose a covalent organic framework (COF)‐based separator with quasi‐single‐ion conduction, specifically a Zn 2+ ‐substituted sulfonate COF (COF‐Zn) membrane, designed to tackle these issues. Featuring a high Zn transference number (0.87) and a thin 25 μm profile, the COF‐Zn separator allows for reduced electrolyte usage (20 μL mg −1 ) while effectively minimizing…

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57
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100%
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Authors

9

Topics & keywords

Keywords
  • Separator (oil production)
  • Electrolyte
  • Anode
  • Conductivity
  • Cathode
  • Membrane
  • Chemical engineering
  • Ion
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