Hierarchical interface engineering for advanced magnesium-based hydrogen storage: synergistic effects of structural design and compositional modification

Interface engineering fundamentally revolutionizes magnesium-based hydrogen storage systems by orchestrating atomic-scale interactions and mass transport pathways through precisely engineered structural architectures and chemical environments. This review presents a paradigm-shifting framework that transcends conventional surface modification approaches, establishing interface engineering as a cornerstone strategy for next-generation hydrogen storage materials. Through sophisticated control of interface architecture - from one-dimensional confined channels that facilitate directional hydrogen diffusion, to two-dimensional platforms that maximize catalytic interactions, to three-dimensional networks that…

• NS
  National Science Foundation

  Awards: CMMI-1261782, 1261782
• NS
  Natural Science Foundation of Chongqing

  Awards: CSTB2024NSCQ-MSX1034, CSTB2024NSCQ
• CS
  Centre Scientifique et Technique du Bâtiment
• NK
  National Key Research and Development Program of China

  Award: 2023YFB3809102
• DO
  Division of Civil, Mechanical and Manufacturing Innovation

  Award: CMMI-1261782